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As part of a legal battle over a French winery they once owned as a couple, she claims he abused them during a flight in 2016.
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She described the abuse on the flight in a cross-complaint she filed in a dispute over their French home and winery, which is separate from their ongoing divorce.
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In 2016, several publications quoted unnamed sources who stated that Mr. Pitt did not abuse his children.
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Pitt's unauthorised spokesperson denied Jolie's allegations and said they were "another rehash that hurts the family."
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Over the past decade, Jolie and Pitt have been divorcing, slowed by contested custody battles and a lawsuit over a French winery that they owned a decade ago, Château Miraval.
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For 12 years, Jolie, 47, and Pitt, 58, were among Hollywood's most prominent couples.
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During the decade they had been dating, they got married in 2014, and Jolie filed for divorce in 2016. A judge granted her divorce in 2019, but custody and financial matters are still pending.
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